I believe the headlamp harness running from the dimmer switch to the radiator support is the same from 60-66. The difference in the headlamp harness going to the bulbs begins after the radiator support. You should be able to just bolt in the other grille, and plug the headlamp harness into the existing bulkhead connector.
The only real difference between the 2 light and 4 light harness is an extra pair of wires running from the high beam filament on the low beam lights to the high beam lights.
I have a 66 gmc, one thing I did was to install relays for low and high beams so the bulbs get plenty of voltage and my poor old headlight switch gets a break, bought halogen bulbs at O'reileys $7.00 each, now I can actually see at night......Kieth