It would be a lot simpler to upgrade to a large single alternator, maybe a 200 amp capacity, or something similar. Check into adapting your existing mounting system to allow you to install an alternator like a tractor-trailer system would run. It's virtually impossible to have too much amperage capacity, as the battery will only accept enough current to charge itself. Once both battery banks are fully charged, the regulator will cut the alternator back to a minimum charge, no matter what the upper current limit might be. When I ran a diesel shop service truck, I had an 8D series 12 volt battery that weighed about 120 pounds, and a 200-amp brushless alternator. My booster cables were made from 1-0 welder cable and would carry over 1,000 amps. Boost-starting a big rig was no problem!
Jerry


"It is better to be silent and be thought a fool than to speak and eliminate all doubt!" - Abraham Lincoln
Cringe and wail in fear, Eloi- - - - -we Morlocks are on the hunt!
There is nothing noble in being superior to your fellow man; true nobility is being superior to your former self. - Ernest Hemingway
Love your enemies and drive 'em nuts!